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Ultrafast dynamics in matter group

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UdynI group
Formation2009
FounderCaterina Vozzi
Founded atMilan, Italy
TypeResearch group
Legal statusActive
HeadquartersIFN-CNR,   Politecnico di Milano
Location
FieldsAttosecond Science,   Ultrafast dynamics
Membership
  • Caterina Vozzi
  • Salvatore Stagira
  • Michele Devetta
  • Eugenio Cinquanta
  • Egle Molotokaite
  • Davide Faccialà
  • Anna Gabriella Ciriolo
  • Gabriele Crippa
  • Matteo Bonanomi
  • Lorenzo Gatto
  • Bogdan Constanin Ispas
  • Stavroula Vovla
  • Andrea Annunziata
Official language
English,   Italian
LeaderCaterina Vozzi
Websiteudyni.eu


The Ultrafast dynamics in matter (UdynI) group is a joint research group between the Istituto di Fotonica e Nanotecnologie of the Italian National Research Council (CNR-IFN) and the Physics Department of Politecnico di Milano. Their research is focused on attosecond science and ultrafast spectroscopy. The group is led by Caterina Vozzi.

Research Activity

Ultrafast THz Spectroscopy
Ultrafast THz Spectroscopy is a state-of-the-art technique that encompasses the study of light-matter interaction with an unprecedented temporal and spatial resolution. Ultrafast means times in the femtosecond and attosecond scale. It revolves around the generation of isolated attosecond light pulses and their phase matching.
Attosecond Science
In Attosecond Science, these aforementioned pulses excite and probe matter on the temporal scales typical of electron dynamics. The sample is excited by two signals, one from the pump exciting carriers in the valence band and one from the probe exciting carriers in core orbitals, with a delay in respect to the first one. The signal is then measured with a spectrometer which produces either absorption or reflectivity spectra.
High Harmonic Generation (HHG) spectroscopy
Pulse generation is based on High-order Harmonic Generation (HHG). HHG is a strongly non-linear optical process which involves the emission of coherent radiation, co-linear to the pump, with a characteristic comb-like spectrum of odd harmonics of the fundamental laser field.

Publications

2020
G. Folpini et al. “Ultrafast charge carrier dynamics in quantum confined 2D perovskite” JOURNAL OF CHEMICAL PHYSICS 152, (2020)
O. Plekan et al. “Experimental and Theoretical Photoemission Study of Indole and Its Derivatives in the Gas Phase” JOURNAL OF PHYSICAL CHEMISTRY A 124, 4115-4127 (2020)
A. G. Ciriolo et al. “High-order harmonic generation in a microfluidic glass device” Journal of Physics: Photonics 2, 024005 (2020)
A. G. Ciriolo et al. “Femtosecond Laser-Micromachining of Glass Micro-Chip for High Order Harmonic Generation in Gases” MICROMACHINES 11, 165 (2020)
T. J. Asel et al. “Influence of Surface Chemistry on Water Absorption in Functionalized Germanane” CHEMISTRY OF MATERIALS 32, 1537-1544 (2020)
M. Mudrich et al. “Ultrafast relaxation of photoexcited superfluid He nanodroplets” NATURE COMMUNICATIONS 11, 112 (2020)
2019
E. Cinquanta et al. “Ultrafast THz Probe of Photoinduced Polarons in Lead-Halide Perovskites” PHYSICAL REVIEW LETTERS 122, 166601 (2019)
2008
A. G. Ciriolo et al. “Generation of ultrashort pulses by four wave mixing in a gas-filled hollow core fiber” J. Opt. 20, 125503 (2018)
J. Mauritsson et al. “Emerging attosecond technologies” J. Opt. 20, 110201 (2018)
M. Negro et al. “Fast stabilization of a high-energy ultrafast OPA with adaptive lenses” Sci Rep 8, 14317 (2018)
S. Bietti et al. “Ga metal nanoparticle-GaAs quantum molecule complexes for terahertz generation” Nanotechnology 29, 365602 (2018)
V. Cardin et al. “Self-channelled high harmonic generation of water window soft x-rays” J. Phys. B-At. Mol. Opt. Phys. 51, 174004 (2018)
D. Facciala et al. “High-order harmonic generation spectroscopy by recolliding electron caustics” J. Phys. B-At. Mol. Opt. Phys. 51, 134002 (2018)
2017
S. L. Cousin et al. “Attosecond Streaking in the Water Window: A New Regime of Attosecond Pulse Characterization” Phys. Rev. X 7, 041030 (2017)
K. Kovacs et al. “Attosecond lighthouse above 100eV from high-harmonic generation of mid-infrared pulses” J. Opt. 19, 104003 (2017)
M. Di Fraia et al. “Impulsive laser-induced alignment of OCS molecules at FERMI” Phys. Chem. Chem. Phys. 19, 19733-19739 (2017)
M. Shcherbinin et al. “Interatomic Coulombic decay in helium nanodroplets” Phys. Rev. A 96, 013407 (2017)
O. Tchulov et al. “Laser induced strong-field ionization gas jet tomography” Sci Rep 7, 6905 (2017)
S. Kuhn et al. “The ELI-ALPS facility: the next generation of attosecond sources” J. Phys. B-At. Mol. Opt. Phys. 50, 132002 (2017)
C. Callegari et al. “Application of Matched-Filter Concepts to Unbiased Selection of Data in Pump-Probe Experiments with Free Electron Lasers” Appl. Sci.-Basel 7, 621 (2017)
C. Vozzi et al. “Tracking the dynamics of electron expulsion” Science 356, 1126 (2017)
A. G. Ciriolo et al. “Optical Parametric Amplification Techniques for the Generation of High-Energy Few-Optical-Cycles IR Pulses for Strong Field Applications” Appl. Sci.-Basel 7, 265 (2017)
M. Ilchen et al. “Circular Dichroism in Multiphoton Ionization of Resonantly Excited He+ Ions” Phys. Rev. Lett. 118, 013002 (2017)
T. Takanashi et al. “Time-Resolved Measurement of Interatomic Coulombic Decay Induced by Two-Photon Double Excitation of Ne-2” Phys. Rev. Lett. 118, 033202 (2017)
2016
D. Iablonskyi et al. “Slow Interatomic Coulombic Decay of Multiply Excited Neon Clusters” Phys. Rev. Lett. 117, 276806 (2016)
D. Facciala et al. “Probe of Multielectron Dynamics in Xenon by Caustics in High-Order Harmonic Generation” Phys. Rev. Lett. 117, 093902 (2016)
F. Calegari et al. “Advances in attosecond science” J. Phys. B-At. Mol. Opt. Phys. 49, 062001 (2016)
K. C. Prince et al. “Coherent control with a short-wavelength free-electron laser” Nat. Photonics 10, 176+ (2016)
C. Vozzi et al. “2015 International Year of Light and beyond” J. Opt. 18, 010201 (2016)
B. D. Bruner et al. “Multidimensional high harmonic spectroscopy of polyatomic molecules: detecting sub-cycle laser-driven hole dynamics upon ionization in strong mid-IR laser fields” Faraday Discuss. 194, 369-405 (2016)
2015
A. Dubrouil et al. “Two-photon resonant excitation of interatomic coulombic decay in neon dimers” J. Phys. B-At. Mol. Opt. Phys. 48, 204005 (2015)
E. Cinquanta et al. “Optical response and ultrafast carrier dynamics of the silicene-silver interface” Phys. Rev. B 92, 165427 (2015)
M. Reduzzi et al. “Advances in high-order harmonic generation sources for time-resolved investigations” J. Electron Spectrosc. Relat. Phenom. 204, 257-268 (2015)
J. Moses et al. “Special issue on optical parametric processes” J. Opt. 17, 090201 (2015)
2014
M. Negro et al. “Non-collinear high-order harmonic generation by three interfering laser beams” Opt. Express 22, 29778-29786 (2014)
H. Soifer et al. “Studying the universality of field induced tunnel ionization times via high-order harmonic spectroscopy” J. Opt. 20, 125503 (2014)
L. Poletto et al. “Spectrometer for X-ray emission experiments at FERMI free-electron-laser” Rev. Sci. Instrum. 85, 103112 (2014)
P. O'Keeffe et al. “Experimental investigation of the interatomic Coulombic decay in NeAr dimers” Phys. Rev. A 90, 042508 (2014)
L. Poletto et al. “Double-configuration grating monochromator for the spectral selection of ultrashort pulses” Appl. Optics 53, 5879-5888 (2014)
M. Negro et al. “High-order harmonic spectroscopy for molecular imaging of polyatomic molecules” CHEMISTRY OF MATERIALS 32, 1537-1544 (2014)
O. Vendrell et al. “Chemical reaction dynamics I and electron dynamics in molecules: general discussion” Faraday Discuss. 171, 145-168 (2014)
2013
D. Shafir et al. “Trajectory-Resolved Coulomb Focusing in Tunnel Ionization of Atoms with Intense, Elliptically Polarized Laser Pulses” Phys. Rev. Lett. 111, 023005 (2013)
F. Frassetto et al. “Active-grating monochromator for the spectral selection of ultrashort pulses” Opt. Express 21, 12996-13004 (2013)
D. Fazzi et al. “Ultrafast spectroscopy of linear carbon chains: the case of dinaphthylpolyynes” Phys. Chem. Chem. Phys. 15, 9384-9391 (2013)
M. Nisoli et al. “Current frontiers of ultrafast and high field optics: Attosecond science” Riv. Nuovo Cimento 36, 105-172 (2013)
2012
B. Mahieu et al. “Full tunability of laser femtosecond high-order harmonics in the ultraviolet spectral range” Appl. Phys. B-Lasers Opt. 108, 43-49 (2012)
F. Calegari et al. “Temporal gating methods for the generation of isolated attosecond pulses” J. Phys. B-At. Mol. Opt. Phys. 45, 074002 (2012)
S. Bonora et al. “Optimization of low-order harmonic generation by exploitation of a resistive deformable mirror” Appl. Phys. B-Lasers Opt. 106, 905-909 (2012)
C. Vozzi et al. “Strong-field phenomena driven by mid-infrared ultrafast sources” J. Mod. Opt. 59, 1283-1302 (2012)
V. Tosa et al. “Isolated Attosecond Pulse Generation by Two-Mid-IR Laser Fields” IEEE J. Sel. Top. Quantum Electron. 18, 239-247 (2012)
2011
M. Negro et al. “Gating of high-order harmonics generated by incommensurate two-color mid-IR laser pulses” Laser Phys. Lett. 8, 875-879 (2011)
C. Vozzi et al. “Generalized molecular orbital tomography” Nat. Phys. 7, 822-826 (2011)
F. Calegari et al. “Quantum path control in harmonic generation by temporal shaping of few-optical-cycle pulses in ionizing media” Phys. Rev. A 84, 041802 (2011)
I. S. Lopez et al. “Local nanotailoring of polymeric photophysics by Au nanoparticles implantation” Cryst. Res. Technol. 46, 833-835 (2011)
C. Vozzi et al. “Phase-matching effects in the generation of high-energy photons by mid-infrared few-cycle laser pulses” New J. Phys. 13, 073003 (2011)
G. Cerullo et al. “Few-optical-cycle light pulses with passive carrier-envelope phase stabilization” Laser Photon. Rev. 5, 323-351 (2011)
S. Coraggia et al. “Carbon coatings for extreme-ultraviolet high-order laser harmonics” Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. 635, S43-S46 (2011)
N. D. Ouart et al. “Analysis of the simultaneous measurements of iron K- and L-shell radiation from ultrashort laser produced plasmas” J. Phys. B-At. Mol. Opt. Phys. 44, 065602 (2011)
2010
C. Vozzi et al. “High harmonic generation spectroscopy of hydrocarbons” Appl. Phys. Lett. 97, 241103 (2010)
F. Ferrari et al. “High-energy isolated attosecond pulses generated by above-saturation few-cycle fields” Nat. Photonics 4, 875-879 (2010)
C. Altucci et al. “Interplay between group-delay-dispersion-induced polarization gating and ionization to generate isolated attosecond pulses from multicycle lasers” Opt. Lett. 35, 2798-2800 (2010)
C. Vozzi et al. “High Order Harmonics Driven by a Self-Phase-Stabilized IR Parametric Source” Laser Phys. 20, 1019-1027 (2010)
M. Negro et al. “Polarization pulse shaping induced by impulsive molecular alignment in optical filamentation and application to high-order harmonic generation” Opt. Lett. 35, 1350-1352 (2010)
T. Virgili et al. “Role of intramolecular dynamics on intermolecular coupling in cyanine dye” Phys. Rev. B 81, 125317 (2010)
C. Vozzi et al. “High-order harmonics generated by 1.5 mu m parametric source” J. Mod. Opt. 57, 1008-1013 (2010)
F. Calegari et al. “Filamentation-assisted time-resolved Raman spectroscopy in molecular gases” J. Mod. Opt. 57, 967-976 (2010)Category:Time-resolved spectroscopy



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